CNRS Associate Researcher in Physico-Chemistry of solid polymers
I am a CNRS researcher focusing on the mechanics of soft and hard polymer networks, and more specifically on how heterogeneous architectures can impact and potentially improve their mechanical and physical response.
I have completed a PhD thesis in Materials Science in the group of Pr. Thomas Pardoen at UCLouvain in Belgium. Then, I have pursued a post-doctoral stay in the group of Pr. Zhigang Suo at Harvard University in the field of Soft Active Materials for two years. As a second postdoc, I worked on the mechanics and fracture of multiple-network elastomers and pressure-sensitive adhesives in the Laboratory of Soft Matter Science and Engineering at ESPCI Paris along with Pr. Costantino Creton and Pr. Matteo Ciccotti. I have now joined the Polymer Materials Engineering Lab (IMP - UMR5223) at INSA-Lyon where I am now building my own research group.
To learn more details on my background, have a look at my CV.
01/2023 : Glad to announce, I’ll have the privilege for this new year to join the editorial board of Engineering Fracture Mechanics Journal as a junior Advisory Board Member.
12/2022 : Go have a quick look at the General audience media section for a small ad on the novel work initiative in medical engineering developped in Lyon around building an artificial organ platform for medical devices validation through the MIMIMed project that I will co-manage with Guilhem Rival (principal project carrier) from LGEF laboratory and Rémy Gauthier from Matéis lab.
11/2022 : Good news with 2 of our papers accepted for publication (see “Publications”) with (i) the work of Benoit Caprin on the rheological and mechanical behavior of thermoreversible physical organo-hydrogels based on polysaccharides, and (ii) the work of Xavi Lacambra Andreu on the characterization and modelling of self-healing process (through macromolecular chain diffusion) occuring during 3D-printing by filament deposition.
10/2022 : Welcome to Barthelemy Gros who joins the IMP lab to start his PhD, co-supervised with Paul Sotta, Jean-François Gérard and myself. He will be focusing on the detection of early damage by nano-cavitation in the polymer liner of hyperbar hydrogen tanks as part of the HYPERSTOCK project insisde the Decarbonated Hydrogen National Consortium #PEPR_H2.
09/2022 : I am happy to announce a new collaboration with Hutchinson Research & Innovation Center who will be funding the master thesis project of Clémence Taffner who will be working on the durability of Fuel cells seals in acidic environment.
06/2022 : Congrats to Loup Mambré who has succesfully secured his funding for a ministry-funded (MESR) PhD after a well-prepared and executed oral defense at the Ecole Doctorale 34 of Lyon! => Enjoy some well-deserved holidays Loup before coming back in the fall to start working on ionic-liquid modified epoxy networks!
keywords : mechanics and fracture of polymer networks, multi-scale characterization, micro-mechanical modeling, design of smart active materials.
A common trait throughout my whole research experience is the strong will of seeking a better molecular understanding of polymer networks deformation and fracture micromechanisms, in order to in-fine establish more clearly the relation between polymer microstructure and their macroscopic properties. Building on the knowledge of this rather theoretical quest, I also envision to tackle more multi-disciplinary and coupled problems through the study and design of soft active materials. The area of soft matter mechanics being extremely vast, it still offers plenty of room for new exciting developments.
Projects : in construction…
# 2020 - now : Laboratoire Ingénierie des Matériaux Polymères (IMP - UMR5223) | INSA de Lyon, Villeurbanne, FRANCE
Prospective research on the large strain and fracture behavior of ionic liquid (IL) modified polymer systems. The first step focuses on controlling the mechanical behavior through the topological nano-structuration of a phosphonium-ionic liquid epoxy system, while in second step multi-functional responses will be also considered, taking advantage of IL conductivity and thermal properties. The work is performed in the laboratoire d’Ingénierie des Matériaux Polymères (IMP) in collaboration with S. Livi & Pr. S. Pruvost.
# 2017 - 2019 : ESPCI | PSL, Paris, FRANCE
Fundamental research using mechano-chemistry as a tool to study the mechanics and fracture of soft polymer networks, going from adhesives to hydrogels and elastomers. A focus is set on the understanding of the stress-transfer and fatigue mechanisms occurring in multiple network hydrogels and elastomers through optical analysis of fluorescent molecular markers. The work is performed in SIMM lab in collaboration with Pr. Creton, Pr. Ciccotti & Pr. Barthel.
# 2015 - 2017 : School of Engineering and Applied Science | Harvard, Cambridge - MA, USA
Research in the field of soft active materials in the group of Pr. Zhigang Suo. My research involved the preparation of tough hydrogels, their specific mechanical and fracture characterization under a large variety of testing conditions (from sub-zero temperatures to fatigue loading), as well as the development of new engineering devices making use of their multifunctional properties.
# 2011 - 2015 : IMAP, iMMC | UCLouvain, Louvain-la-Neuve, BELGIUM
Research in materials science with both experimental and modeling work in the field of mechanics of polymers and polymer-based composites. Development of an original physics-based theory for modelling the meso-scale heterogeneous micro-mechanisms of glassy polymers. Collaborations on applied research projects with the aeronautical industry (Safran group, TechSpace Aero, Sonaca), as well as fundamental research with other international groups (KULeuven, Trinity College, IMDEA, Imperial College), were pursued in parallel.
Dissertation: “Mechanical Characterization and Physics-Based Modeling of a Highly-Crosslinked Epoxy Resin”, supervised by Pr. Thomas Pardoen \& Pr. Christian Bailly.
# 2010 - 2011 : Erasmus student exchange in the Chemical Engineering and Chemistry Department | TU/e Eindhoven University of Technology, Eindhoven, NETHERLANDS
Five months stay as a visiting master student, including a two-months research project in the field of nano-composites under the supervision of Pr. L.E. Govaert and Pr. J.G.P. Goosens.
2023
2022
2021
DEPOS, co-presented keynote talk with Pr. Sylvie Castagnet - FRA - September 29th : Mécanismes de cavitation dans des élastomères sous décompression d’hydrogène : apports de la tomographie in-situ et de la mécanochimie
EURADH 2021 Virtual meeting, keynote session - FRA - October 12th : Role of damage by sacrificial bonds: Intrinsic differences between fatigue and toughness mechanisms in multiple network elastomers.
UMass, Polymer Science and Engineering, Crosby research group - virtual webinar (Amherst, MA, USA) - March 24th: Mechanochemistry as a tool to study cavitation in multiple network elastomers.
2020
2019
University of Amsterdam, Soft Matter Group, Van der Walls-Zeeman Institute (Institute of Physics) - Amsterdam - NED - November 28th: 3D Visualization of cavitation process in multiple network elastomers.
ESPCI - SIMM lab thematic workshop on Soft Matter Mechanics, Paris - FRA - November 13th : 3D Visualization of cavitation process in multiple network elastomers.
APS (American Physical Society) March meeting, Boston (MA) - USA - March 6th : Towards a unified model of soft adhesives (on behalf of Matteo Ciccotti).
University of Michigan, Ann-Arbor (MI) - USA - February 27th : From the meso-scale modeling of epoxy resins to the fatigue of hydrogels: a micro-mechanical approach of polymer networks.
Universidade do Porto, Porto - POR - January 28th: Macroscopic viscoplastic behavior of thermosets - RTM6 as a case study.
2018
pre-print works
xx. X. P. Morelle, J. Chopin, C. Creton, E. Barthel, M. Ciccotti, “Critical parameters governing heterogeneous adhesion of PSA on textured surfaces”, under preparation.
yy. R. Bai, X. P. Morelle, J. Wang, Z. Suo, “Rupture and debonding of soft layered materials”, under preparation.
2022
B. Caprin, G. Viñado-Buil, G. Sudre, X. P. Morelle, F. Da Cruz-Boisson, A. Charlot, and E. Fleury, “κ‐Carrageenan Associated with Fructose/Glycerol/Water LTTM: Toward Natural Thermosensitive Physical Gels”, ACS Sustainable Chemistry & Engineering, 2022. https://doi.org/10.1021/acssuschemeng.2c04437
X. Lacambra Andreu, X. P. Morelle, Abderrahim Maazouz, Jean-Marc Chenal, and Khalid Lamnawar,”Rheological investigation and modeling of healing properties during extrusion-based 3D printing of poly(lactic-acid)”,accepted in Rheologica Acta, *2022.
2021
X. Yao, B. Chen, X. P. Morelle, Z. Suo, “Anti-icing propylene glycol materials”,Extreme Mechanics Letters, 2021, vol 44, 101225. https://doi.org/10.1016/j.eml.2021.101225.
T. Pardoen, N. Klavzer, S. Gayot, F. Van Loock, J. Chevalier, X. P. Morelle, V. Destoop, F. Lani, P. Camanho, L. Brassart, B. Nysten, C. Bailly, “Nanomechanics serving polymer-based composite research”, Comptes Rendus de Physique,for the “Plasticity and Solid State Physics” special issue, 2021.doi:10.5802/crphys.56
H. Chabane, S. Livi, X. P. Morelle, Rodolphe Sonnier, Loïc Dumazert, Jannick Duchet-Rumeau, Jean-François Gérard, “Synthesis of New Ionic Liquid-Grafted Metal-Oxo Nanoclusters – Design of Nanostructured Hybrid Organic-Inorganic Polymer Networks”, Polymer for “GFP 50th Anniversary” special issue, 2021. https://doi.org/10.1016/j.polymer.2021.123721
X. P. Morelle, G. E. Sanoja, S. Castagnet, C. Creton, “3D Fluorescent Mapping of Invisible Molecular Damage after Cavitation in Hydrogen Exposed Elastomers”, Soft Matter, 2021. https://doi.org/10.1039/D1SM00325A
G. E. Sanoja, X. P. Morelle, J.Comtet, C. Creton, “Why is Mechanical Fatigue Different from Toughness in Elastomers? The Role of Damage by Polymer Chain Scission”, 2021, Science Advances, pre-print available on ChemRxiv.
2019
2018
J. Chevalier#, L. Brassart, F. Lani, C. Bailly, T. Pardoen, X. P. Morelle#, “Unveilling the nanoscale heterogeneity controlled deformation of thermosets”, Journal of the Mechanics and Physics of Solids, vol 121, 2018, pp. 432-446. https://doi.org/10.1016/j.jmps.2018.08.014
X. P. Morelle, W. R. Illeperuma, K. Tian, R. Bai, Z. Suo, J. J. Vlassak, “Highly stretchable and tough hydrogels below water freezing temperatures”, Advanced Materials, vol 30, 2018, 1801541. https://doi.org/10.1002/adma.201801541
P. Rothemund, X. P. Morelle, K. Jia, G. M. Whitesides, Z. Suo, “A transparent membrane for active noise cancelation”, Advanced Functional Materials, vol 28, 2018, 1800653. https://doi.org/10.1002/adfm.201800653
E. Zhang, R. Bai, X. P. Morelle, Z. Suo, “Fatigue fracture of nearly elastic hydrogels”, Soft Matter, vol 14, 2018, pp. 3563-3571. https://doi.org/10.1039/C8SL00460A
R. Bai, J. Yang, X. P. Morelle, C. Yang, Z. Suo, “Fatigue fracture of self-recovery hydrogels”, ACS Macro Letters, vol 7, 2018, pp. 312-317. https://doi.org/10.1021/acsmacrolett.8b00045
2017
X. P. Morelle, R. Bai, Z. Suo, “Localized deformation in Plastic Liquids on Elastomers”, Journal of Applied Mechanics, vol. 84 : issue 10, 2017, pp. 101002 https://doi.org/10.1115/1.4037410
R. Bai, Q. Yang, J. Tang, X. P. Morelle, J. Vlassak, Z. Suo, “Fatigue fracture of tough hydrogels”, Extreme Mechanics Letters, vol 15, 2017, pp. 91-96. https://doi.org/10.1016/j.eml.2017.07.002
X. P. Morelle, J. Chevalier, C. Bailly, T. Pardoen, F. Lani, “Mechanical characterization and modeling of the deformation and failure of the highly crosslinked RTM6 epoxy resin”, Mechanics of Time-Dependent Materials, vol. 21 : issue 3, 2017, pp. 419-454. https://doi.org/10.1007/s11043-016-9336-6
2016
J. Chevalier, X. P. Morelle, C. Bailly, P.P. Camanho, T. Pardoen, F. Lani, “Micro-mechanics based pressure dependent failure model for highly cross-linked epoxy resin”, Engineering Fracture Mechanics, vol. 158, 2016, pp.192-216. https://doi.org/1016/j.engfracmech.201602.039
V.-D. Nguyen, F. Lani, T. Pardoen, X. P. Morelle, L. Noels, “A large strain hyperelastic viscoelastic-viscoplastic-damage constitutive model based on a multi-mechanism non-local damage continuum for amorphous glassy polymers”, International Journal of Solids and Structures, vol. 96, 2016, pp. 192-216. https://doi.org/10.1016/j.ijsolstr.2016.06.008
2015
Invited lecturer for a 2h seminar on the viscoplasticity of polymers, given to an auditorium of 50 engineering students in their 2nd year of master degree.
Preparation and monitoring of lab sessions (2h/week) with a brief theoretical course before actual experiments given to 50 engineering students in their 1st year of master degree. T.A. also involved the correction and grading of lab reports. Topic : lab #1 (Deformation and fracture at the macro-scale - uniaxial tension test and stress-strain curves); lab #2 (Introduction to fracture and concept of toughness - Critical stress intensity factor (K1c) computation.
Monitoring exercises sessions (4h/week) of classes of 30 students in 1st year of bachelor in engineering. Topic : Atomic structure, intra- and inter-molecular bounds and associated properties; introduction to thermodynamics (concepts of enthalpy, heat, entropy, spontaneous and non-spontaneous processes); acid-base reactions.
Monitoring excercise and lab session (2h/week + 6h of lab) of classes of 20 students in 2nd year of bachelor in engineering. Topic : Perfect gases, kinetic theory of gases; 1st (closed and open systems) and 2nd principle of thermodynamics ; chemical equilibrium between gaseous and aqueous phases; applications to electro-chemistry and redox reactions.
post-graduate level (4) not in dissertation commitee : mentoring and collaborative work with Xavi Lacambra (2021-2022) at INSA-Lyon, Louis Debertrand (2018-2019) at ESPCI, Jérémy Chevalier (2015-2018) at UCLouvain, and Ruobing Bai (2016-2017) at Harvard University.
graduate level (7) : daily based supervision of master students thesis project (6 months to 1 year) : Noémie Maamouri & Joanna Baudino (2021, materials science, INSA-lyon), Ana-Carolina Fernandez Rodas (2021, materials science, INSA-lyon), Elina Gilbert (2019, materials science, ESPCI), Loïc Van Nieuwenhuyse (2014-2015, materials science, UCL), Minh Le Duy (2013-2014, macromolecular nanotechnology, UCL), Jesus Gutierrez Martinez (2012-2013, mechanical engineering, UCL).
undergrad level (3) : co-supervision of 2 to 6 month research internship of : Emmanuel Fabing (2022, INSA-Lyon), Ana Santos (2018, ESPCI) and Enrui Zhang (2016, Harvard University).
Group seminar organizer for the IMP lab (2020-current) - Organization of internal group seminars for exposing the work of PhD studends, post-docs and permanent researchers, in order to promote exchanges and collaborations between lab members.
Mechanical Testing equipment trainer in INSA-Lyon site of the IMP lab (2019-current) - Person-in-charge for new training on Uniaxial testing machines (Instron and MTS) for quasi-static, fracture and fatigue loading of polymer-based specimens.
Lab visit and science promotion for teenagers in SIMM lab at ESPCI Paris (2017-2019) - Organization of small lab visit and experimental demonstration for high school students during occasional week-long science camps.
Trustee in the board of directors of Gravelines rowing club (2017-now) - As a trustee, I get involved into the general management, planning and new projects development of Gravelines rowing club. My missions non exhaustively include the organization and participation to international rowing regattas, preparation of the annual general membership meeting, and promotion of the club activities on social networks.
Lab safety officer and equipment trainer in Suo Lab at Harvard University (2016-2017) - Emergency lab contact, development of equipment safety procedure, LN2 ordering, chemical inventory and waste disposal coordination. Person-in-charge for new training on Instron testing machine and on the high-voltage amplifier.
Board member of Harvard-MIT Belgian Society in Boston (2016-2017) - Organizing social networking events and open debates among the belgian community (and more) in the Boston area, in order to promote Belgian scientific, political or economical personalities and achievements.
New equipment purchase and installation for Suo Lab installation at Harvard University (2016) - Purchase of a universal testing machine with associated load cells and temperature chamber. Coordination of lab duct work and machine installation with Harvard McKay building teams.
co-organizer of the PhD promotion day at iMMC, UCLouvain (2011-2014) - Lab promotion presentation and visit organized for 2nd year engineering master students.
Student representative at EPL, UCLouvain (2008-2011) - Involvement within the Applied Physics and Chemistry degree program commission and work with academic authorities. Coordinate and organize examination schedule as well as other extra-academic group activities.
12/2022 : quick youtube presentation of the pluri-disciplinary work initiative in medical engineering developped in Lyon through the Carnot Institut funding and more specifically of the MIMIMed project aiming at building an artificial organs platform for pre-clinical validation of medical devices.
12/2020 : article of Johanna Miller from Physics Today on the use of mechano-fluorescent molecular probes to study the fracture of elastomers, highlighting the work performed in the group of Costantino Creton these last years and in particular the thesis of Juliette Slootman. Stretchy molecules rupture far from the crack
05/2019 : Following my talk at the APS March Meeting conference, a journalist (Ryan F. Mandelbaum) from the the American online science journal Gizmodo contacted Pr. Matteo Ciccotti and wrote a nice article explaining some of the motivations and results of our group’s work on adhesion of pressure sensitive adhesives. Scientists Are Stuck on the Mystery of Tape
07/2017 : Daily Science article on Belgian scientists abraod (FR) : Matériaux intelligents et régates à Harvard